Harry Potter Cruciatus Curse. After Harry sacrificed himself in the Forest none of Voldemorts spells worked including the Cruciatus Curse. The Cruciatus Curse Crucio also known as the Torture Curse was a tool of the Dark Arts and one of the three Unforgivable Curses.
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Shortly afterwards Harry cast the Cruciatus Curse on him for spitting in Professor McGonagalls face DH30. Using it on any human being is punished lifelong imprisonment at Azkaban. Interestingly the magical government saw fit to allow its own employees the Aurors to freely employ these three spells against anyone associated with Death Eaters during the First Wizarding War.
It is one of the most powerful and sinister spells known to wizardkind.
Bartemius Crouch II Tom Riddle. It was one of the most powerful and sinister spells known to Wizardkind. The Unforgivable Curses in Harry Potter Imperio Crucio and Avada Kedavra are considered the three worst spells known to wizardkind and were supposedly penalized with the worst possible punishment in 1717. The Cruciatus Curse also known as the Torture Curse Crucio is a tool of the Dark Arts and one of the three Unforgivable Curses.